Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene (Springer Theses)
Language: English
Published by Springer, 2017
- Hardcover
- New
Seller: California Books, Miami, FL, U.S.A.California Books
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- Title
- Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene (Springer Theses)
- Author
- Hou, Ruijun
- Publisher
- Springer
- Publication year
- 2017
- Condition
- New
- Binding
- Hardcover
- Language
- English
- ISBN 10
- 9811007721
- ISBN 13
- 9789811007729
- Series
- Book 238 of 797: Springer Theses
This thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd–Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD). The excellent correlation between model surfaces and supported catalysts demonstrates the feasibility of designing effective bimetallic catalysts for selective hydrogenation reactions. The author also proposes a method for designing non-precious metal catalysts to replace precious metals. She modifies the process of selective hydrogenation of acetylene by coupling the selective adsorption to the selective hydrogenation in the liquid phase, as a result of which the ethylene selectivity is greatly improved and heat transfer is greatly enhanced. Lastly, by analyzing the mechanism of liquid-phase hydrogenation, the author proposes a multi-stage slurry bed reactor for industrial applications.<
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California Books
Miami, FL, U.S.A.
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