Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene
Language: English
Published by Springer Singapore, 2017
- Hardcover
- New
Condition: New
£ 79.56
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Dieser Artikel ist ein Print on Demand Artikel und wird nach Ihrer Bestellung fuer Sie gedruckt. Nominated by Tsinghua University as an outstanding Ph.D. thesisReports on important advances in catalysis for selective hydrogenationCombines theoretical and experimental research to deliver a novel method for catalyst designProvides.
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- Title
- Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene
- Author
- Ruijun Hou
- Publisher
- Springer Singapore
- Publication year
- 2017
- Condition
- New
- Binding
- Gebunden
- Language
- English
- ISBN 10
- 9811007721
- ISBN 13
- 9789811007729
- Series
- Book 238 of 797: Springer Theses
This thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd–Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD). The excellent correlation between model surfaces and supported catalysts demonstrates the feasibility of designing effective bimetallic catalysts for selective hydrogenation reactions. The author also proposes a method for designing non-precious metal catalysts to replace precious metals. She modifies the process of selective hydrogenation of acetylene by coupling the selective adsorption to the selective hydrogenation in the liquid phase, as a result of which the ethylene selectivity is greatly improved and heat transfer is greatly enhanced. Lastly, by analyzing the mechanism of liquid-phase hydrogenation, the author proposes a multi-stage slurry bed reactor for industrial applications.<
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