Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene
Language: English
Published by Springer Nature Singapore, Springer Nature Singapore, 2017
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- New
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- Title
- Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene
- Author
- Ruijun Hou
- Publisher
- Springer Nature Singapore, Springer Nature Singapore
- Publication year
- 2017
- Condition
- Neu
- Binding
- Buch
- Language
- English
- ISBN 10
- 9811007721
- ISBN 13
- 9789811007729
- Item weight
- 407 grams
- Dimensions
- 241x160x15 mm
- Series
- Book 238 of 797: Springer Theses
This thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd–Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD). The excellent correlation between model surfaces and supported catalysts demonstrates the feasibility of designing effective bimetallic catalysts for selective hydrogenation reactions. The author also proposes a method for designing non-precious metal catalysts to replace precious metals. She modifies the process of selective hydrogenation of acetylene by coupling the selective adsorption to the selective hydrogenation in the liquid phase, as a result of which the ethylene selectivity is greatly improved and heat transfer is greatly enhanced. Lastly, by analyzing the mechanism of liquid-phase hydrogenation, the author proposes a multi-stage slurry bed reactor for industrial applications.<
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